Polarization control of metal-enhanced fluorescence in hybrid assemblies of photosynthetic complexes and gold nanorods
文献信息
Ł. Bujak, M. Olejnik, T. H. P. Brotosudarmo, M. K. Schmidt, N. Czechowski, D. Piatkowski, J. Aizpurua, R. J. Cogdell, W. Heiss, S. Mackowski
Fluorescence imaging of hybrid nanostructures composed of a bacterial light-harvesting complex LH2 and Au nanorods with controlled coupling strength is employed to study the spectral dependence of the plasmon-induced fluorescence enhancement. Perfect matching of the plasmon resonances in the nanorods with the absorption bands of the LH2 complexes facilitates a direct comparison of the enhancement factors for longitudinal and transverse plasmon frequencies of the nanorods. We find that the fluorescence enhancement due to excitation of longitudinal resonance can be up to five-fold stronger than for the transverse one. We attribute this result, which is important for designing plasmonic functional systems, to a very different distribution of the enhancement of the electric field due to the excitation of the two characteristic plasmon modes in nanorods.
期刊推荐

Bioorganic & Medicinal Chemistry

Journal of the Indian Institute of Science

Journal of Asian Natural Products Research

Colloid Journal

Critical Reviews in Solid State and Materials Sciences

Acta Metallurgica Sinica-English Letters

Topics in Catalysis

Journal of Chemical Sciences

Chinese Journal of Chemistry

Polycyclic Aromatic Compounds
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Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.



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