Whirl-enhanced continuous wave laser trapping of particles‡
文献信息
S. Bartkiewicz, A. Miniewicz
Tightly focused laser beams can trap micro- and nanoparticles suspended in liquids in their focal spots enabling different functionalities including 3D manipulations and assembling. Here, we report on remarkably strong liquid–liquid phase separation and crystallization experiments in para-nitroaniline dissolved in 1,4-dioxane. For optical trapping of para-nitroaniline we used low-power, weakly focused light beam from continuous-wave laser partially absorbed by the solute. The experiments were performed in solution deposited on glass with an upper free-surface and solution contained between two glass plates. The usual gradient force field and scattering force solely are insufficient to properly describe the observed particle gathering effects extending far beyond the optical trap potential. The concept of whirl-enhanced and temperature assisted optical trapping is postulated. The relative simplicity of the used geometry for trapping will broaden the understanding of the light-matter interaction and promises the widespread application of the observed effect in optically controlled crystallization.
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来源期刊
Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.













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