Self-assembled systems for artificial photosynthesis
文献信息
Sebastiano Campagna, Francesco Nastasi, Giuseppina La Ganga, Scolastica Serroni, Antonio Santoro, Antonino Arrigo, Fausto Puntoriero
The last few decades have seen an impressive development in molecular-based artificial photosynthesis, thanks to the design of integrated light-harvesting antennae, charge separation systems, and catalysts for water oxidation or hydrogen production based on covalently linked subunits. However, in recent years, self-assembly and spontaneous aggregation of components emerged – sometimes also through serendipity – for the preparation of multicomponent systems aimed to perform the basic processes needed for artificial photosynthesis. Here we critically discuss some key articles that have recently shown the potential of self-assembly for artificial photosynthesis, ranging from self-assembly of antennae and charge separation systems to integrated antenna/catalyst assemblies, to planned co-localization of various components into restricted environments. It is evident that self-assembly can generate emerging properties with respect to the non-aggregated species, and such emerging properties can be quite convenient for designing efficient photocatalytic systems.
相关文献
Synthesis and field-effect transistor properties of a diseleno[3,2-b:2′,3′-d]silole-based donor–acceptor copolymer: investigation of chalcogen effect
Yu-Chieh Pao, Cheng-Tai Yang, Yu-Ying Lai, Wen-Chia Huang, Chain-Shu Hsu, Yen-Ju Cheng
DOI: 10.1039/C6PY00765A
Bioinspired synthesis of poly(phenylboronic acid) microgels with high glucose selectivity at physiological pH
Qingshi Wu, Xue Du, Aiping Chang, Xiaomei Jiang, Xiaoyun Yan, Xiaoyu Cao, Zahoor H. Farooqi, Weitai Wu
DOI: 10.1039/C6PY01521B
Chiral fluorescent sensors based on cellulose derivatives bearing terthienyl pendants
Tomoyuki Ikai, Daisuke Suzuki, Yutaka Kojima, Changsik Yun, Katsuhiro Maeda, Shigeyoshi Kanoh
DOI: 10.1039/C6PY00967K
Synthesis of a glucose oxidase-conjugated, polyacrylamide-based, fluorescent hydrogel for a reusable, ratiometric glucose sensor
Ho Namgung, Taek Seung Lee
DOI: 10.1039/C6PY01120A
An amphiphilic block copolymer conjugated with carborane and a NIR fluorescent probe for potential imaging-guided BNCT therapy
Zheng Ruan, Le Liu, Liyi Fu, Tao Xing, Lifeng Yan
DOI: 10.1039/C6PY00799F
Reductive triblock copolymer micelles with a dynamic covalent linkage deliver antimiR-21 for gastric cancer therapy
Changyu He, Zhen Zhang, Qinglai Yang, Qing Chang, Zhifeng Shao, Yu-Mei Shen, Bingya Liu, Zhenggang Zhu
DOI: 10.1039/C6PY00651E
Mechanical properties of single supramolecular polymers from correlative AFM and fluorescence microscopy
M. F. Knopper
DOI: 10.1039/C6PY01656A
Facile synthesis and the properties of novel cardo poly(arylene ether sulfone)s with pendent cycloaminium side chains as anion exchange membranes
Ruiqiang Wang, Xinbing Chen, Pei Chen, Zhongwei An, Suobo Zhang
DOI: 10.1039/C7PY00690J
您可能还喜欢
甲基双烯双酮(CAS号:5173-46-6)通常如何合成?
甲基双烯双酮可以通过多种途径合成。一种常见的合成方法是通过甲基化和环化反应,先由4-甲基-9-烯-1,3-二酮合成,然后进行环化反应得到目标产物。具体的合成路线...
如何处理含有tert-butyl 3,5-difluorobenzoate(CAS号:467442-11-1)的废料?
处理含有tert-butyl 3,5-difluorobenzoate(CAS号:467442-11-1)的废液时,应首先收集并密封,避免泄漏。随后,建议通过焚...
4-二甲氧基甲基-2-(三氟甲基)嘧啶(CAS号:878760-47-5)通常如何合成?
4-二甲氧基甲基-2-(三氟甲基)嘧啶通常通过三氟甲基化反应合成。首先,将2-氯嘧啶与三氟甲基锂在惰性溶剂中反应,然后将得到的三氟甲基化中间体与二甲氧基甲基化试...
WRW4(CAS号:878557-55-2)的主要用途是什么?
WRW4主要应用于科学研究领域,尤其是在合成化学和有机合成方面。由于其特殊的化学性质,它可能被用于特定的化学反应或合成过程。
什么是6-O-(三异丙基硅基)-D-葡萄烯糖(CAS号:137915-37-8)?
6-O-(三异丙基硅基)-D-葡萄烯糖是一种有机化合物,化学名为1,5-Anhydro-2-deoxy-6-O-(triisopropylsilyl)-D-ar...
N-Benzyl-N,N-dimethyl-2-phenoxyethanaminium(CAS号:7181-73-9)的主要用途是什么?
N-Benzyl-N,N-dimethyl-2-phenoxyethanaminium在有机合成中被用作保护基团,可以用于保护氨基,提高反应的选择性和产率。此外...
什么是3-(Cyclohex-1-en-1-yl)acrylic acid(CAS号:56453-88-4)?
3-(Cyclohex-1-en-1-yl)acrylic acid,简称3-环己烯-1-烯丙酸,是一种含有环己烯基团的丙烯酸衍生物,用于合成其他化合物或作为有...
如何储存(1R)-7-fluoro-1,2,3,4-tetrahydronaphthalen-1-amine(CAS号:1055949-62-6)?
应将(1R)-7-氟-1,2,3,4-四氢萘胺储存于阴凉、干燥、通风良好的地方,远离火源和热源。避免与氧化剂、酸类接触。使用合适的容器,密封保存。
3-甲基苯并呋喃-2-羧酸(CAS号:24673-56-1)的主要用途是什么?
3-甲基苯并呋喃-2-羧酸主要用作合成其他化合物的中间体,如药物合成、有机合成等领域。此外,该化合物在某些领域作为化学试剂或分析试剂使用。
孕烷醇酮(CAS号:128-20-1)适用哪些法规指南?
孕烷醇酮(CAS号:128-20-1)需遵守GHS(全球化学品统一分类和标签制度)的相关分类和标签要求,主要涉及健康危害、环境危害和物理化学危害。此外,还需要遵...
来源期刊
Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.










![2-[2-(2-Methoxyethoxy)ethoxy]-2-methylpropane structure 2-[2-(2-Methoxyethoxy)ethoxy]-2-methylpropane structure](https://cnstatic.chemtradehub.com/structs/527/52788-79-1-71c1.webp)


![2-Bromo-7-chloro-4H-pyrrolo[2,3-b]pyrazine structure 2-Bromo-7-chloro-4H-pyrrolo[2,3-b]pyrazine structure](https://cnstatic.chemtradehub.com/structs/115/1150617-58-5-0b0a.webp)
