A rational guide to improve the activity of a hydrogen-evolving polymeric carbon nitride photocatalyst

文献信息

发布日期 2023-11-21

DOI 10.1039/D3SE00996C

影响因子 6.367

作者

Tomoharu Maeda, Chomponoot Suppaso, Shunta Nishioka, Yoshinobu Kamakura, Shuhei Yasuda, Toshiyuki Yokoi

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摘要

Photocatalytic H2 evolution using Pt-loaded mesoporous polymeric carbon nitride (meso-PCN) was studied with respect to light intensity and the hydrogen窶電euterium isotope effect, in combination with photoelectrochemical measurements. Although the photocatalytic activity was mainly limited by charge recombination in the meso-PCN, improving the oxidation reaction by photogenerated holes was critical for enhancing the H2-evolution activity. The finding of this work will be a useful guide to achieve non-sacrificial overall water splitting by PCN photocatalysts.

期刊推荐

Journal of Heterocyclic Chemistry

Molecular Pharmacology

Science Progress

Journal of Organometallic Chemistry

Pure and Applied Chemistry

Kinetics and Catalysis

Planta Medica

Journal of Physics and Chemistry of Solids

Fibre Chemistry

Proceedings of the National Academy of Sciences of the United States of America

来源期刊

Sustainable Energy & Fuels

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自引率: 0%

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A rational guide to improve the activity of a hydrogen-evolving polymeric carbon nitride photocatalyst

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来源期刊

Sustainable Energy & Fuels

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