Steps, hops and turns: examining the effects of channel shapes on mass transfer in continuous electrochemical reactors

文献信息

发布日期 2022-01-06
DOI 10.1039/D1RE00530H
影响因子 4.239
作者

Hamish R. Stephen, Sarah Boyall, Christiane Schotten, Richard A. Bourne, Nikil Kapur, Charlotte E. Willans


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摘要

Due to the heterogenous nature of electrochemical reactions, mass transport is an important consideration during reaction and reactor development. The effect of different flow channel geometries on mass transfer between wall and solution within a continuous electrochemical reactor has been investigated using experimental studies and computational fluid dynamics. The channel shape is shown to have modest impact on the mass transfer coefficient. However, the reaction solution hopping from one side of an electrode to the other, so switching polarity mid-flow, has the greatest effect.

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来源期刊

Reaction Chemistry & Engineering

Reaction Chemistry & Engineering
CiteScore: 0
自引率: 8.8%
年发文量: 284

Reaction Chemistry & Engineering is an interdisciplinary journal reporting cutting-edge research focused on enhancing the understanding and efficiency of reactions. Reaction engineering leverages the interface where fundamental molecular chemistry meets chemical engineering and technology. Challenges in chemistry can be overcome by the application of new technologies, while engineers may find improved solutions for process development from the latest developments in reaction chemistry. Reaction Chemistry & Engineering is a unique forum for researchers whose interests span the broad areas of chemical engineering and chemical sciences to come together in solving problems of importance to wider society. All papers should be written to be approachable by readers across the engineering and chemical sciences. Papers that consider multiple scales, from the laboratory up to and including plant scale, are particularly encouraged.

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